Search results for "gas cell"

showing 10 items of 14 documents

Offline commissioning of a new gas cell for the MARA Low-Energy Branch

2023

Results of offline commissioning tests for a new dedicated gas cell for the Mass Analysing Recoil Apparatus (MARA) Low-Energy Branch are reported. Evacuation time, ion survival and transport efficiency in helium buffer gas were characterized with a radioactive 223Ra 𝛼-recoil source. Suppression of the ion signal, originating from non-neutralized species in the gas cell, was explored with 219Rn ions, the daughter recoil of 223Ra, as a function of voltage applied to one of the ion-collector electrodes. Two-step laser resonance ionization of stable tin isotopes produced inside the gas cell from a heated bronze filament was demonstrated, and broadening of the atomic resonances in argon buffer …

223Ra α-recoil sourceNuclear and High Energy Physicstutkimuslaitteetgas cellin-gas laser ionizationydinfysiikkaInstrumentationMARA-LEBNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Opportunities and limitations of in-gas-cell laser spectroscopy of the heaviest elements with RADRIS

2022

International audience; The radiation detection resonance ionization spectroscopy (RADRIS) technique enables laser spectroscopic investigations of the heaviest elements which are produced in atom-at-a-time quantities from fusion-evaporation reactions. To achieve a high efficiency, laser spectroscopy is performed in a buffer-gas environment used to thermalize and stop the high-energy evaporation residues behind the velocity filter SHIP. The required cyclic measurement procedure in combination with the applied filament collection for neutralization as well as confinement of the stopped ions and subsequent pulse-heat desorption constrains the applicability of the technique. Here, some of these…

Actinidesactinideslaser spectroscopygas celltutkimusmenetelmätSuper heavy elements[PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det]Laser spectroscopy[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]laserspektroskopiasuper heavy elementsGas cell
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Developments towards in-gas-jet laser spectroscopy studies of actinium isotopes at LISOL

2015

To study exotic nuclides at the borders of stability with laser ionization and spectroscopy techniques, highest efficiencies in combination with a high spectral resolution are required. These usually opposing requirements are reconciled by applying the in-gas-laser ionization and spectroscopy (IGLIS) technique in the supersonic gas jet produced by a de Laval nozzle installed at the exit of the stopping gas cell. Carrying out laser ionization in the low-temperature and low density supersonic gas jet eliminates pressure broadening, which will significantly improve the spectral resolution. This article presents the required modifications at the Leuven Isotope Separator On-Line (LISOL) facility…

ActiniumNuclear and High Energy PhysicsRocket engine nozzleSeparator (oil production)chemistry.chemical_elementactinium[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]7. Clean energy01 natural sciencesResonance ionization spectroscopylaw.inventionAtmospheric-pressure laser ionizationlawIonization0103 physical sciencesPhysics::Atomic Physics[PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det]010306 general physicsSpectroscopyInstrumentationGas jetJet (fluid)ta114010308 nuclear & particles physicsChemistrygas cellLaserActiniumresonance ionization spectroscopygas jetAtomic physicsGas cellNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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Gas cell studies of thorium using filament dispensers at IGISOL

2020

Abstract Filament-based dispensers of thorium have been investigated at the IGISOL facility, Jyvaskyla, for potential use as a thorium ion source for future collinear laser spectroscopy experiments. Several different filaments were manufactured in the Institute of Atomic and Subatomic Physics of TU Wien, with 232Th and 229Th prepared on tantalum substrates either by drying thorium nitrate solution or via molecular plating, while adding a layer of zirconium for oxide reduction. The filaments were characterized in a helium-filled gas cell by performing selective and efficient in-gas-cell resonance laser ionization and by analyzing the resulting ion beams by mass spectrometry. Additionally, th…

DECOMPOSITIONNuclear and High Energy PhysicsTechnologyEFFICIENCYAnalytical chemistrychemistry.chemical_elementOFF-LINEPhysics Atomic Molecular & ChemicalMass spectrometry01 natural sciencesIonlaw.inventionProtein filamentlawIonization0103 physical sciences010306 general physicsNuclear Science & TechnologyLANTHANIDEInstrumentationInstruments & InstrumentationRESONANCE IONIZATIONScience & TechnologySPECTROSCOPYResonance laser ionization010308 nuclear & particles physicsPhysicsThoriumThoriumLASER ION-SOURCEActinideLaserIon sourceIon sourceWORK-FUNCTIONSPhysics NuclearchemistryACTINIDE ELEMENTSPhysical SciencesGas cellTRANSITION
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Characterization of a cryogenic ion guide at IGISOL

2012

A small volume cryogenic ion guide has been characterized at the IGISOL facility, Jyvaskyla, as a prototype to verify whether there are any major obstacles to the use of high-density cryogenic helium gas for the stopping and extraction of high-energy ions from a large volume cryogenic ion catcher. The expected temperature scaling of the mass flow through the ion guide has been confirmed, showing that for the same helium density, the differential pumping requirements are less stringent for cryogenic operation. At 90 K a clear reduction in the mass-analyzed impurities is achieved, although lower temperatures are required to freeze out oxygen and nitrogen. This is supported by the reduction in…

EXTRACTIONNuclear and High Energy PhysicsDISSOCIATIVE RECOMBINATIONOrders of magnitude (temperature)Mass flowCryogenic gas cellONLINEchemistry.chemical_elementPRESSURENOIonIon beam depositionELECTRON-TEMPERATURE DEPENDENCEASSOCIATION REACTIONSRadioactive ion beamsInstrumentationHeliumDissociative recombinationIon guidePhysicsta114Volume (thermodynamics)chemistryGASAtomic physicsBeam (structure)HELIUMNuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment
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Rate capability of a cryogenic stopping cell for uranium projectile fragments produced at 1000 MeV/u

2016

At the Low-Energy Branch (LEB) of the Super-FRS at FAIR, projectile and fission fragments will be produced at relativistic energies, separated in-flight, energy-bunched, slowed down and thermalized in a cryogenic stopping cell (CSC) filled with ultra-pure He gas. The fragments are extracted from the stopping cell using a combination of DC and RF electric fields and gas flow. A prototype CSC for the LEB has been developed and successfully commissioned at the FRS Ion Catcher at GSI. Ionization of He buffer gas atoms during the stopping of energetic ions creates a region of high space charge in the stopping cell. The space charge decreases the extraction efficiency of stopping cells since the …

Nuclear and High Energy PhysicsEXTRACTIONFissionBuffer gasION-CATCHER01 natural sciencesSpace chargeIonHEAVY-IONSNuclear physicsMOBILITIESElectric fieldIonization0103 physical sciencesRate capabilityddc:530SPECTROMETER010306 general physicsNuclear ExperimentInstrumentationSUPER-FRSHIGH-PRECISION EXPERIMENTSta114010308 nuclear & particles physicsChemistryProjectileBEAMSPERFORMANCEGAS CELLSpace chargeExtraction efficiencyExtraction timeCryogenic gas-filled stopping cellAtomic physicsBeam (structure)Nuclear Instruments & Methods in Physics Research Section B-Beam Interactions with Materials and Atoms
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Advancing Radiation-Detected Resonance Ionization towards Heavier Elements and More Exotic Nuclides

2022

Atoms 10(2), 41 (2022). doi:10.3390/atoms10020041

Nuclear and High Energy Physicsatomic level schemeresonance ionizationgas celllaser spectroscopylaser spectroscopy; resonance ionization; atomic level scheme; gas cell; radiation detection; heavy actinidesddc:530radiation detectionCondensed Matter Physics530heavy actinidesAtomic and Molecular Physics and Optics
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Observation of Collisional De-Excitation Phenomena in Plutonium

2022

Proceedings for the "virtual Workshop on the Atomic Structure of Actinides & Related Topics" conference submitted to the special issue of Atoms "Atomic Structure of the Heaviest Elements". A program of research towards the high-resolution optical spectroscopy of actinide elements for the study of fundamental nuclear structure is currently ongoing at the IGISOL facility of the University of Jyväskylä. One aspect of this work is the development of a gas-cell-based actinide laser ion source using filament-based dispensers of long-lived actinide isotopes. We have observed prominent phenomena in the resonant laser ionization process specific to the gaseous envir…

Nuclear and High Energy Physicscollisional de-excitationplutoniumactinidetutkimuslaitteetgas cellCondensed Matter PhysicsAtomic and Molecular Physics and Opticsgas-cellcollisional de-excitation; actinide elements; resonance laser ionization; gas cellresonance laser ionizationlaser resonance ionizationPhysics::Atomic Physicsactinide elementsNuclear ExperimentydinfysiikkaAtoms
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In-gas-cell laser ionization studies of plutonium isotopes at IGISOL

2016

Abstract In-gas-cell resonance laser ionization has been performed on long-lived isotopes of Pu at the IGISOL facility, Jyvaskyla. This initiates a new programme of research towards high-resolution optical spectroscopy of heavy actinide elements which can be produced in sufficient quantities at research reactors and transported to facilities elsewhere. In this work a new gas cell has been constructed for fast extraction of laser-ionized elements. Samples of 238–240,242 Pu and 244 Pu have been evaporated from Ta filaments, laser ionized, mass separated and delivered to the collinear laser spectroscopy station. Here we report on the performance of the gas cell through studies of the mass spec…

Nuclear and High Energy PhysicsplutoniumAnalytical chemistrychemistry.chemical_element01 natural sciences7. Clean energylaw.inventionlawIonization0103 physical sciencesPhysics::Atomic PhysicsNuclear Experiment010306 general physicsSpectroscopyInstrumentationHeliumArgonta114010308 nuclear & particles physicsgas cellActinideLaserPlutoniumchemistryresonance laser ionizationMass spectrumgas phase chemistryNuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
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First Offline Results from the S3 Low-Energy Branch

2022

International audience; We present the first results obtained from the S3 Low-Energy Branch , the gas cell setup at SPIRAL2-GANIL, which will be installed behind the S3 spectrometer for atomic and nuclear spectroscopy studies of exotic nuclei. The installation is currently being commissioned offline, with the aim to establish optimum conditions for the operation of the radio frequency quadrupole ion guides, mass separation and ion bunching, providing high-efficiency and low-energy spatial spread for the isotopes of interest. Transmission and mass-resolving power measurements are presented for the different components of the S3-LEB setup. In addition, a single-longitudinal-mode, injection-lo…

Nuclear and High Energy Physicsresonance ionization laser spectroscopy; gas cell; hypersonic gas jets; radio frequency quadrupoles; nuclear ground state properties; isotope shift; hyperfine structurehyperfine structurespektroskopiatutkimuslaitteet[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]Physics Atomic Molecular & Chemicalatomifysiikka[PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det]radio frequency quadrupolesScience & TechnologySPECTROSCOPY[PHYS.PHYS.PHYS-ATOM-PH]Physics [physics]/Physics [physics]/Atomic Physics [physics.atom-ph]Physicsgas cellLASER ION-SOURCECondensed Matter PhysicslasertekniikkaAtomic and Molecular Physics and Opticsresonance ionization laser spectroscopyisotope shiftnuclear ground state propertiesPhysical Scienceshypersonic gas jetsIONIZATIONydinfysiikkaSYSTEMAtoms
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